Hi Kelli, great question! You should be able to, yes, but you'll need to make sure the Spotify app is installed on your Gear Sport. You can also pair Bluetooth headphones directly with that watch, so that may be another option to explore. You can do that by going to Settings > Connections > Bluetooth on the watch, then selecting "BT headset" while your headset is in pairing mode. Then just select the headset, and you should be good to go! ^Matthew